2D Materials, Volume (8), No (3), Year (2021-7)

Title : ( Role of charge doping and strain in the stabilization of in-plane ferromagnetism in monolayer VSe2 at room temperature )

Authors: Sara Memarzadeh , Mahmood Rezaee Roknabadi , Mohsen Modarresi , Aybey Mogulkoc , Aleksandar Rudenko ,

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Abstract

We study the origin of in-plane ferromagnetism in monolayer VSe2 focusing on the effect of charge doping and mechanical strain. We start from an anisotropic spin Hamiltonian, estimate its parameters from density functional calculations, and determine the spectrum of spin-wave excitations. We show that 1T-VSe2 is characterized by relatively strong on-site Coulomb repulsion (U sime 5 eV), favoring an antiferromagnetic ground state, which contradicts experimental observations. We calculate the magnetic phase diagram as a function of charge doping and strain, and find a transition to the ferromagnetic state with in-plane easy axis under moderate hole doping (~1014 cm−2). Analysis of spin-wave excitations in doped monolayer VSe2 reveals a gap due to the in-plane anisotropy, giving rise to long-range magnetic order well above 300 K, in agreement with recent experiments. Our findings suggest that experimentally available 1T-VSe2 monolayer samples might be intrinsically or extrinsically doped, which opens up the possibility for a controllable manipulation of their magnetic properties.

Keywords

, VSe2 monolayer, Ferromagnetism
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@article{paperid:1084788,
author = {Memarzadeh, Sara and Rezaee Roknabadi, Mahmood and Modarresi, Mohsen and Aybey Mogulkoc and Aleksandar Rudenko},
title = {Role of charge doping and strain in the stabilization of in-plane ferromagnetism in monolayer VSe2 at room temperature},
journal = {2D Materials},
year = {2021},
volume = {8},
number = {3},
month = {July},
issn = {2053-1583},
keywords = {VSe2 monolayer; Ferromagnetism},
}

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%0 Journal Article
%T Role of charge doping and strain in the stabilization of in-plane ferromagnetism in monolayer VSe2 at room temperature
%A Memarzadeh, Sara
%A Rezaee Roknabadi, Mahmood
%A Modarresi, Mohsen
%A Aybey Mogulkoc
%A Aleksandar Rudenko
%J 2D Materials
%@ 2053-1583
%D 2021

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